Browse Topic: Nylon

Items (200)
Researchers have developed a solar-powered reactor to break down hard-to-recycle forms of plastic waste – such as drinks bottles, nylon textiles and polyurethane foams – using acid recovered from old car batteries, and converting it into clean hydrogen fuel and valuable industrial chemicals.
Polypropylene, a commodity plastic, is the semi-crystalline thermoplastics widely used in high volume for general purpose application. Polypropylene is the macro molecules of soft and weak backbone, which by reinforcement of fillers in different forms such as fiber, spheroids, nanotubes, flakes, etc., can influence its mechanical, thermal, electrical, creep resistance, and flame resistance properties for use in aerospace applications. Currently, polycarbonate and nylon plastics are used in aerospace applications, however, they are expensive compared with polypropylene. In this thesis, efforts are put to study the effect of reinforcement fillers in the properties of polypropylene composite, primarily the mechanical and flammability properties. The matrix element, polypropylene co polymer and reprocessed polypropylene blended in equal ratio, are coupled with the dispersing phases such as graphene, mica, fumed silica, and polydimethylsiloxane polymer. Effect of graphene as reinforcing filler at different weight % to polypropylene composite’s properties are studied and compared with that of the neat polypropylene. Effect of coupling agent, Aminopropyltriethoxysilane (APTES), on mineral fillers and Polydimethylsiloxane polymer (PDMS) used for crosslinking with the polypropylene matrix is also studied and compared using Fourier Transform Infrared Spectroscopy (FTIR) and Scanning Electron Microscope (SEM) techniques.
Govindaraju, Parthasarathy
Certain materials — such as quartz, some ceramics, and even bone — produce an electrical charge when they are squeezed, pressed, or vibrated. This is piezoelectricity, which comes from the Greek “piezein” meaning to press. Modern vehicles rely on piezo components in fuel injectors, parking sensors, airbag systems, and other functions.
Automotive industry frequently uses 3D printed plastic proto parts during new product development phases as it bypasses the high tooling investment & development time at early part development stage. However, for some application, 3D printing technique & its limited material options are not fulfilling the required material properties in the part, resulting poor performance during product testing which may mislead the design engineer during validation process. To overcome this, we introduce a novel approach in constructing injection molding tool by 3D printing the core and cavity using Stereolithography (SLA). This enables production of parts with application-recommended material grades, facilitating traditional validation and increasing stakeholder confidence. This paper compares part quality from 3D printed molds against conventional metallic molds for a shifter gear housing cover, demonstrating a 45% reduction in tooling costs and a 75% decrease in tooling development time. Mold life analysis using PP Glass Filled 30% (PPGF30) and Nylon 66 Glass Filled 30% (Nylon 66GF30) yielded approximately 100 and 25 parts, respectively. We also discussed the challenges encountered during the mold 3D printing and injection molding process. This innovative technique offers broad applicability across plastic part manufacturing industries.
Gandhi, Sorna RajendranGunduboina, Chaitanya
The automotive industry leverages Fused Filament Fabrication (FFF) -based Additive Manufacturing (AM) to reduce lead time and costs for prototypes, rapid tooling, and low-volume customized designs. This paper examines the impact of print orientation and raster angle on the tensile properties of Polylactic Acid (PLA), selected for its ease of use and accessibility. Dog bone samples were designed to the ASTM D638 tensile testing standard and printed solid with a 0.2 mm layer height, two outer walls, and varying raster-fill angles, with layers alternating by 90°. Testing was conducted on the MTS Criterion Model 43, 50 kN system. Varying print orientation along the X and Y axes (double angle builds) produced a Young's modulus (YM) range of 0.7519, reflecting a 34.42% increase between the witnessed minimum and maximum values. These builds exhibited more brittle behavior than most single angle builds, except for X10 Y10 Z0 at a 45° raster (the lowest recorded YM) and X0 Y15 Z0 at a 30° raster (the highest recorded YM). The same build orientation (X0 Y15 Z0) with varying raster angles between 0°-90° resulted in a yield stress range between 2.53 and 3.31 kN/mm2. These findings show that strategic build parameter configuration enables PLA to exhibit both flexible and rigid characteristics. Therefore, when creating AM solutions, Design for Additive Manufacturing (DfAM) and material selection are important, but slicing parameters also play a crucial role in determining a part's final mechanical properties. These findings lay the groundwork for applying this experiment methodology to other thermoplastics commonly used in the automotive industry, such as ABS and Nylons. This research aims to provide detailed experimental data, highlighting extreme values and uncertainties in the tensile strength of FFF samples. Understanding how build orientation influences part strength can help engineers optimize performance and predict failure modes.
Strelkova, DoraUrbanic, Ruth Jill
Friction stir welding (FSW) is a method of welding that creates a weld trail by pressing a non-consumable rotating tool with a profiled pin on the adjacent surfaces while moving transversely along the welding direction. The method was initially used with metals and alloys, but more recently, thermoplastic polymers have also been included in its application. Investigations on FSW of thermoplastic polymers made of nylon and High-density polythene (HDPE) are presented here. Weld characteristics that are like those of the base materials are attempted to be achieved. Because of their unique nature and thermal conductivity, thermoplastics FSW differs from that of metals. The use of thermoplastic materials with conventional FSW procedures presents numerous difficulties and is currently ineffective. On the weld characteristics of nylon and HDPE, statistical methods were utilized to study the impact of temperature, rotational speed, and transverse speed. Temperature is found to be the most important factor, followed by rotational and traversal speeds. In general, a higher temperature in combination with lower transverse speeds produced the most desirable results. Nylon exhibited a higher UTS of 35MPa when compared with HDPE which possess UTS of 16.7 MPa after friction stir welding under optimized process parameters with using induction assisted coil. A welding efficiency of 55% and 41% were observed for nylon and HDPE respectively based on their base material UTS. Microstructural aspects will also be discussed.
Raju, GangaChinnakurli Suryanarayana, RameshSrivastava, Ashish
G-3, Aerospace Couplings, Fittings, Hose, Tubing Assemblies
Nylon polymer with an optimal blend of Kevlar, fiberglass, and high-speed, high temperature (HSHT) Fiberglass offers improved characteristics such as flexural strength, wear resistance, electrical insulation, shock absorption, and a low friction coefficient. For this reason, the polymer composite manufactured by combining HSHT, Kevlar, and fiberglass with nylon as base material will expand the uses of nylon in the aerospace, automotive, and other industrial applications related to ergonomic tools, assembly trays, and so forth. The proposed work was carried out to investigate the continuous fiber reinforcement (CFR) in nylon polymer using a dual extrusion system. Twenty experimental runs were designed using a face-centered central composite design (FCCD) approach to analyze the influence of significant factors such as reinforcement material, infill pattern, and fiber angle on the fabricated specimen as per American Society for Testing Materials (ASTM) standards. The tensile strength, percentage elongation, and surface roughness of each test specimen (ASTM) have been investigated using the universal testing machine (UTM) and a surface roughness tester. A set of regression equations connecting process input factors and output features have been derived using the response surface methodology (RSM). In addition, the MOGA-ANN method is employed to achieve the multi-response targets. The results show that the best tensile strength and surface roughness are achieved with a 64.5-degree fiber angle, fiberglass CFR, and a triangular infill pattern, while the best balance and optimal response are achieved with a 49.2575-degree fiber angle, a rectangular fill pattern, and fiberglass reinforcement using the MOGA-ANN evolutionary hybrid algorithm. With MOGA-ANN, the least surface roughness of 1.43158 microns, maximum tensile strength, and percentage elongation of 37.869 MPa and 51.05% were attained at these parameters, and the same has been validated experimentally.
Kaushik, AshishKumar, PardeepGahletia, SumitGarg, Ramesh KumarKumar, AshishYadav, MohitGiri, JayantChhabra, Deepak
This specification covers the requirements for nonperforated nylon paper base plastic honeycomb core material for aircraft structural applications, including exterior parts such as radio and radar antenna housings.
AMS P17 Polymer Matrix Composites Committee
In this study the volume and hardness were measured for thermoplastics and thermosetting resins with diesel containing up to 30% of the following blend stocks: biodiesel, renewable diesel, n-undecane, dibutoxymethane, 1-octanol, hexyl hexanoate, and 2-nonanone. Thermoplastics included polyphenylene sulfide (PPS), polyethylene terephthalate (PET), polytetrafluoroethylene (PTFE), polyvinylidene fluoride (PVDF), polyoxymethylene (POM), polybutylene terephthalate (PBT), polypropylene (PP), high density polyethylene (HDPE), nylons, acetals, polyetherimide (PEI), polyetheretherketone (PEEK), a PET co-polymer, polyphthalamides (PPAs), polyarylamide (PARA) and ethylene tetrafluoroethylene (ETFE). Three thermosetting resins were also evaluated. The material specimens were exposed to the test fuels under ambient conditions for 16 weeks. In general, the volume and hardness of the specimens were relatively unaffected following exposure to the test fuels; however, n-undecane produced significant swelling in polypropylene and may not be suitable for use with this material. N-undecane, along with hexyl hexanoate and 2-nonanone also caused low levels of swelling in nylon, which was not significant enough to preclude the use of nylons in sealing applications with these fuels.
Kass, MichaelJanke, ChrisNafziger, Eric
Researchers have developed a method that converts cotton into sugar that in turn can be turned into spandex, nylon, or ethanol.
This SAE Standard covers complete general and dimensional specifications for tube fittings of the spherical and flanged sleeve compression types for use in the piping of air brake systems on automotive vehicles. The spherical sleeve compression type Figures 1A to 5 and Tables 1 to 3 is intended for use with annealed copper alloy tubing per SAE J1149, Type 1. The flanged sleeve compression type Figures 6A to 11 and Tables 4 to 6 is intended for use with nylon tubing per SAE J844. It is not intended to restrict or preclude other designs of a tube fitting for use with SAE J844, air brake tubing. Performance requirements for SAE J844 are covered in SAE J1131. See SAE J1131 for the Performance Requirements of Reusable (Push to Connect) Fittings Intended for Use in Automotive Air Brake Systems. CAUTION: To assure satisfactory performance, tapered sleeve compression type fitting components (SAE J512) should not be intermixed with the spherical or flanged sleeve components, nor should the spherical sleeve compression type components be intermixed with the flanged sleeve compression type components when assembling connection in areas where the three types are available.
Air Brake Tubing and Tube Ftg Committee
The compatibilities of fuel system elastomers and plastics were evaluated for test fuels containing 16 vol.% isobutanol (iBu16) and 10 vol.% ethanol (E10). Elastomers included two fluorocarbons, four acrylonitrile butadiene rubbers (NBRs), and one type of fluorosilicone, neoprene, and epichlorohydrin/ethylene oxide. Plastic materials included four nylon grades, three polyamides, polytetrafluoroethylene (PTFE), polyvinylidene fluoride (PVDF), ethylene tetrafluoroethylene (ETFE), polyphenylene sulfide (PPS), high-density polyethylene (HDPE), polybutylene terephthalate (PBT), polyoxymethylene (POM), flexible polyvinylchloride (PVC), polyetherimide (PEI), polyetheretherketone (PEEK), and a phenol formaldehyde reinforced with glass fiber (GFPF). For each polymer material, the volume, mass, and hardness were measured before and after drying. Dynamic mechanical analysis (DMA) measurements were also performed on the dried specimens. For the elastomer materials the measured properties were similar for both fuels. The fluorocarbons and fluorosilicone swelled the least (~20%), while more moderate (20-45%) expansion occurred for the two NBR hose grades and (ECO). HNBR, neoprene, and silicone exhibited high swelling and softening, which likely precludes their use in many fuel systems. For the plastic materials, the observed swell was low; Nylon 11 swelled around 15%, but otherwise, their measured swell was <10%. Many of the plastics also showed sensitivity to alcohol type, as the E10 test fuel often imparted appreciably higher swell than iBu16. In general, the plastic materials showed good compatibility with the iBu16 and E10 test fuels. The sole exception was the PVC material, which was structurally degraded from exposure to either fuel type. Compositional analysis showed high fuel retention in Nylon 12 and PVC. PVC also experienced a significant reduction in plasticizer compounds following exposure, which resulted in embrittlement and an increase in the glass-to-rubber transition temperature.
Kass, MichaelJanke, ChristopherConnatser, Raynella M.Lewis, SamuelBaustian, JamesWolf, LesKoch, Wolf
Fuel efficiency improvement in automobiles has been a topic of great interest over the past few years, especially with the introduction of the new CAFE 2025 standards. Although there are multiple ways of improving the fuel efficiency of an automobile, lightweighting is one of the most common approaches taken by many automotive manufacturers. Lightweighting is even more significant in electric vehicles as it directly affects the range of the vehicle. Amidst this context of lightweighting, the use of composite materials as alternatives to metals has been proven in the past to help achieve substantial weight reduction. The focus of using composites for weight reduction has however been typically limited to major structural components, such as BiW and closures, due to high material costs. Secondary structural components which contribute approximately 30% of the vehicle weight are usually neglected by these weight reduction studies. This work is an attempt to prove that composites can also be used effectively in the weight reduction of secondary structural components, while meeting the desired standards on mechanical performance, cost, and scalability. Discontinuous fiber-reinforced injection-molded materials offer excellent mechanical properties and very high lightweighting potential. In this paper, a secondary structural component such as outside mounted rearview mirror assembly is used to study the effect of performance and cost while trying to achieve a mass reduction of at least 30%. An injection-molded long carbon fiber-reinforced nylon is used to replace the aluminum structure in the baseline mirror assembly. In addition to material replacement, 20%-parts consolidation was achieved due to the design freedom offered by these materials. A virtual plant layout was developed to determine the cost of series manufacturing. In conclusion, this paper provides a strong case for the use of these material systems to lightweight small and secondary structural components.
Ramesh, Senthil RajYerra, Veera AdityaPradeep, Sai AdityaPilla, Srikanth
In recent years, the emerging technology competitions in automotive industry are improving engine efficiency and electronizing for coping with stringent fuel-economy regulations. However, fuel-economy technologies such as engine down-sizing and numerous electronic parts entrust burden plastic materials acing as mainly electric insulation and housing to have to be higher performance, especially temperature endurance. Engineering plastics (EPs) have critical limitations in terms of degradation by heat. Heat-resisting additives in EP are generally used to be anti-degradation as activating non-radical decomposition of peroxide. However, it could not be effective way to impede the degradation in long term heat aging over 1,000 hours at high temperature above 180 °C. In this study, we suggested the new solution called ‘shield effect’ that is purposeful oxidation at the surface and local crystallization of EP to stop prevent penetrating oxygen to inside of that. Ethylene diamine tetra acetic acid (EDTA) and Citric acid (CA) are used as additives for surface oxidation. We added the EDTA and CA to Nylon co-polymer of PA6T/6I-PA66 and made test specimens. Surprisingly, physical properties maintained 5% under degradation rate at 250 °C, over 1,000 hours in contrast with Nylon added general additives. We confirmed surface oxidation and local crystallization of the Nylon by using Energy Dispersive X-ray Spectroscopy (EDX) and X-ray Diffraction Spectroscopy (XRD). Base on this result, we adopt the new materials to high temperature needed automotive parts in engine such as Battery Fuse Terminal (BFT) and Multi Fuse Terminal (MFT), in exhaust system such as Muffler.
Kweon, KyoungchunKim, Seong Jin
The guarantee of long-term reliability of cars is becoming increasingly important in society. It is extremely important to confirm whether the condition of the accelerated deterioration test (for evaluating long-term reliability) is reasonable with respect to recent use environment conditions. In this paper, we propose how to promote degradation test conditions to guarantee the function of parts (resin materials of interior parts) exposed over a long period of time to a severe temperature environment inside the car. Heat-resisting grade nylon 66 fiber (hereinafter referred to as H-PA 66), which is a constituent material of parts requiring long-term reliability, was used as a specific resin material. High-temperature accelerated deterioration test of H-PA 66 fiber was carried out to obtain the time (hereinafter referred to as 90% strength time,) during which the tensile strength retention rate decreased to 90%. The relationship between this high temperature accelerated deterioration temperature and 90% intensity time could be expressed by the Arrhenius equation. The acceleration rate of deterioration was determined from the Arrhenius plot of this equation. At the same time, we propose DOE (Design of Engineering) graph which can judge deterioration by expressing accelerated deterioration temperature on the vertical axis and accelerated deterioration time on the horizontal axis. We predicted deterioration after 15 years from the temperature history of the actual environment obtained by the exposure test. Moreover, reasonable promotion deterioration condition without excess or deficiency in the case of 15 year guarantee was sought. The DOE graph (capable of expressing the relationship between the actual use environment and accelerated deterioration test condition) improves the accuracy and reliability of the accelerated deterioration condition.
Fukuda, TakeruKai, TakeshiNakada, MasayukiMiyano, YasushiTAJIMA, Yusuke
The compatibility of key fuel system infrastructure plastics with 39 bio-blendstock fuel candidates was examined using Hansen solubility analysis. Fuel types included multiple alcohols, esters, ethers, ketones, alkenes and one alkane. These compounds were evaluated as neat molecules and as blends with the gasoline surrogate, dodecane, and a mix of dodecane and 10% ethanol (E10D). The plastics included polyphenylene sulfide (PPS), polyethylene terephthalate (PET), polytetrafluoroethylene (PTFE), polyvinylidene fluoride (PVDF), polyoxymethylene (POM), polybutylene terephthalate (PBT), polypropylene (PP), high density polyethylene (HDPE), along with several nylon grades. These materials have been rigorously studied with other fuel types, and their volume change results were found to correspond well with their predicted solubility levels. The compatibility was assessed using Hansen solubility parameters and in many instances peak solubility occurred for blends rather than the neat fuel components. The results showed that good compatibilities can be expected for PPS, PVDF, PET, nylons, acetal, PEI, PVC, HDPE and PBT. PTFE showed potential incompatibilities at low blend concentrations, especially when E10D was used as the base fuel blend. Although, the nylons show good overall compatibility, the results do indicate that mid-range and high alcohol contents may not be suitable for Nylon 6 and Nylon 11 in applications requiring low volume swell. Poor potential compatibility was limited to two plastic types; PETG exposed to mid and high blend levels of the ethers and PP exposed to sabinene and the aromatics. In general, the data showed good compatibility for the majority of the candidate fuels and plastics.
Kass, MichaelWest, Brian H.
This SAE Standard covers complete general and dimensional specifications for tube fittings of the spherical and flanged sleeve compression types for use in the piping of air brake systems on automotive vehicles. The spherical sleeve compression type Figures 1A to 5 and Tables 1 to 3 is intended for use with annealed copper alloy tubing per SAE J1149, Type 1. The flanged sleeve compression type Figures 6A to 11 and Tables 4 to 6 is intended for use with nylon tubing per SAE J844. It is not intended to restrict or preclude other designs of a tube fitting for use with SAE J844, air brake tubing. Performance requirements for SAE J844 are covered in SAE J1131. See SAE J1131 for the Performance Requirements of Reusable (Push to Connect) Fittings Intended for Use in Automotive Air Brake Systems. CAUTION: To assure satisfactory performance, tapered sleeve compression type fitting components (SAE J512) should not be intermixed with the spherical or flanged sleeve components, nor should the spherical sleeve compression type components be intermixed with the flanged sleeve compression type components when assembling connection in areas where the three types are available.
Air Brake Tubing and Tube Ftg Committee
Traditionally, Knee Air Bag (KAB) is constructed of a woven nylon or polyester fabric. Recently, Ford developed an injection molded air bag system for the passenger side called Active Glove Box (AGB). This system integrates a plastic bladder welded between the glove box outer and inner doors. This new system is smaller and lighter, thus improving the roominess and other creature comforts inside the passenger cabin while providing equivalent restraint performance as traditional knee airbag system. This patented technology allows positioning of airbags in new locations within the vehicle, thus giving more freedom to designers. The first application of this technology was standard equipment on the 2015 Ford Mustang. Given that this technology is first in the industry, it was a challenge to design, test and evaluate the performance of the system as there is no benchmark to compare this technology. A CAE driven design methodology was chosen to overcome this challenge. This method gave engineers the ability to use an iterative approach to the design and the ability to analytically evaluate the performance of the system. Once a final design was validated through CAE, parts were manufactured and put through physical testing to qualify the design. Quantitative performance of the AGB was then correlated back to CAE results. The CAE prediction shows good correlation to the physical tests. Final design tweaking was performed on the Active Glove Box system to meet the crash safety and other performance requirements.
Lu, LiWest, SeanRaines, StaceyZhou, JinHoke, PaulTay, Yi Yang
This SAE Recommended Practice provides a system for classification and specification for limited number of polyamides (nylons) used in the Automotive Industry. Based upon ASTM D 4066, Classification System for Nylon Injection and Extrusion Materials (PA), it calls for additional descriptive characteristics and properties commonly used in the Automotive Industry. This document applies to natural and non-color matched black, heat-stabilized polyamide compounds only. Color matched compounds shall be defined by the proprietary OEM standards. This document allows for the use of recycled, reconstituted, and regrind materials provided that the requirements as stated in this document are met, the material has not been altered or modified to change its suitability for safe processing and use, and the material shall be identified as such.
Plastics Committee
Microalgae as feedstock are the potential third generation biofuels. Microalgae are photosynthetic microorganism which requires light, carbon-di-oxide, nitrogen, phosphorous, and potassium for growth and to produce lipids, proteins and carbohydrates in large amounts over short a periods of time. The production of biofuels from microalgal is a viable alternative due to their easy adaptability to growth conditions, possibility of growing biomass either in fresh or marine waters. Hence the current project was designed to elucidate the biodiesel producing ability of blue-green algae such as Spirulina platensis and Green algae Chlorella vulgaris. The selected algae were cultivated in suitable growth media such as modified Zarrouke medium and bold basal medium, respectively. The Spirulina platensis and Chlorella vulgaris were mass cultured for 8 days then harvested using 50 micron nylon filters and dried in sunlight to obtain dry biomass. The dried microalgal biomass was extracted for bio-oil production. The extracted bio-oil was analyzed in gas chromatography mass spectrometer (GCMS) to derive its fatty acid profile. From the results, it is clear that 60oC temperature was optimum for bio-oil extraction. The bio-oil thus extracted was converted to biodiesel by trans-esterification process using methanol and NaOH. The quality parameters such as density, viscosity, flash point, iodine value, sulphur and water content of the obtained biodiesel were analysed and found to be in correlation with the EN-14214 standards. From the experiment results it was clear that the yield and analysis parameters of biodiesel were comparatively better in Chlorella vulgaris (75%). The biodiesel extracted from dried biomass of Chlorella vulgaris was tested in 3-cylinder naturally aspirated diesel engine with blend of 20%. Performance and emission parameters have been measured and analysed in this paper.
Nagarajan, RJain, AatmeshVora, Kamalkishore
Samples of 33% glass filled and unfilled poly(butylene terephthalate) [PBT] and nylon 66 (PA66) were injection molded into bars,which were immersed in common engine and powertrain fluids: antifreeze, motor oil and automatic transmission fluid for 25 days. Fluid uptake was measured at 1, 7, 18, and 25 days by gravimetry. Both PBT samples absorbed 0.2-0.25% antifreeze and 0.05 - 0.10% motor oil and automatic transmission fluid (ATF). Both DSC and DMA analysis showed no disruption of polymer thermal transitions or storage moduli. The glass filled PA66 sample absorbed 2.5% antifreeze and 0.25-0.3% of motor oil and ATF and showed an 80°C reduction in the tan delta maximum on DMA. The unfilled PA66 sample absorbed 7% antifreeze and 0.2-0.3% of motor oil and ATF also showed a tan delta maximum 80°C less than the unexposed control. Creep analysis was conducted on the unfilled nylon sample and compared to a virgin material. The softer antifreeze-exposed sample had the expected higher instantaneous strain; however, it had a much reduced viscoelastic response and less permanent deformation. This behavior was thought to arise from hydrogen bond crosslinking of the chains by the imbibed ethylene glycol.
Smith, Robert A.Rudzinskas, Christopher
Creation of a structural joint for a heat shield for extreme entry environments requires structural fibers penetrating through the thickness of the shield at joint locations. The structural fibers must be made of carbon to withstand extremely high temperatures, i.e. 2000 ºC. Carbon fibers, due to their relatively high modulus (stiffness), are easily damaged and broken when handled by a conventional sewing machine. Special coatings such as nylon are required to increase the durability of the fiber to enable its use in a sewing or tufting process.
The compatibility of plastic materials used in fuel storage and dispensing applications was determined for an off-highway diesel fuel and a blend containing 20% bio-oil (Bio20) derived from a fast pyrolysis process. Bio20 is not to be confused with B20, which is a diesel blend containing 20% biodiesel. The feedstock, processing, and chemistry of biodiesel are markedly different from bio-oil. Plastic materials included those identified for use as seals, coatings, piping and fiberglass resins, but many are also used in vehicle fueling systems. The plastic specimens were exposed to the two fuel types for 16 weeks at 60°C. After measuring the wetted volume and hardness, the specimens were dried for 65 hours at 60°C and then remeasured to determine extent of property change. A solubility analysis was performed to better understand the performance of plastic materials in fuel blends composed of bio-oil and diesel. All of the plastic materials evaluated in this study exhibited higher solubility (volume swell) with the Bio20 fuel blend. This result was predicted by the solubility analysis. However, there were two notable exceptions; the volume swell results for high density polyethylene (HDPE) and polypropylene (PP) did not correlate with their respective solubility curves. HDPE and PP were also unique in that they were the only two plastics that exhibited pronounced volume expansion in the baseline diesel test fuel. The plastic materials which showed the best compatibility to the bio-oil blend were the barrier plastics polypropylene sulfide (PPS), polyethylene terephthalate (PET or Mylar™), and polytetrafluoroethylene (PTFE or Teflon™). Polyvinylidene fluoride (PVDF or Kynar™) is also used extensively as a permeation barrier material; however, it swelled over 15% when exposed to Bio20. Four grades of nylon were evaluated and the petroleum-derived nylons (Nylon 6, Nylon 6,6, and Nylon 12) showed good compatibility with the test fuels. In contrast, Nylon 11, which is derived from vegetable oil, expanded over 4% with Bio20. HDPE also swelled around 4%, but did so with both test fuels. Two acetal materials and polybutylene terephthalate (PBT) were also observed to swell to 4% with Bio20. Four fiberglass resins were included in the study and they exhibited 10-18% volume expansion. High volume swell was also noted for PP, the PET polyethylene - glycol copolymer (PETG), and polythiourea (PTU). PP also expanded over 15% following exposure to the baseline diesel test fuel.
Kass, Michael D.Janke, ChrisConnatser, RaynellaLewis, SamKeiser, JamesTheiss, Timothy
The compatibility of plastic materials used in fuel storage and dispensing applications was determined for a test fuel representing gasoline blended with 10% ethanol. Prior investigations were performed on gasoline fuels containing 25, 50 and 85% ethanol, but the knowledge gap existing from 0 to 25% ethanol precluded accurate compatibility assessment of low level blends, especially for the current E10 fuel (gasoline containing 10% ethanol) used in most filling stations, and the recently accepted E15 fuel blend (gasoline blended with up to15% ethanol). For the majority of the plastic materials evaluated in this study, the wet volume swell (which is the parameter most commonly used to assess compatibility) was higher for fuels containing 25% ethanol, while the volume swell accompanying E10 was much lower. However, several materials, such as polyvinylidene fluoride (PVDF), fiberglass resins, and the polyethylene terephthalate co-polymer (PETG) exhibited similar volume expansions with both 10 and 25% ethanol. In the second part of this study, the compatibility performance of the infrastructure plastics in the E10 test fuel was compared to a test fuel containing 16% isobutanol (which has the same oxygen level as E10). The measured property changes (volume and hardness) in these two fuels were similar for the majority of the plastics tested. However, Nylon 6, Nylon 6,6, and the vinyl ester fiberglass resin showed much better compatibility with a 16% isobutanol blend than with a blend containing 10% ethanol.
Kass, Michael D.Janke, ChrisTheiss, TimothyBaustian, JamesWolf, LeslieKoch, Wolf
The compatibility of plastic materials used in gasoline storage and dispensing applications was determined for test fuels representing neat gasoline (Fuel C), and blends containing 25% ethanol (CE25a), 16% isobutanol (CiBu16a), and 24% isobutanol (CiBu24a). A solubility analysis was also performed and compared to the volume swell results obtained from the test fuel exposures. The plastic specimens were exposed to each test fuel for16 weeks at 60°C. After measuring the wetted volume and hardness, the specimens were dried for 65 hours at 60°C and then remeasured for volume and hardness. Dynamic mechanical analysis (DMA), which measures the storage modulus as a function of temperature, was also performed on the dried specimens to determine the temperature associated with the onset of the glass-to-rubber transition (Tg). For many of the plastic materials, the solubility analysis was able to predict the relative volume swell for each test fuel. Those plastic materials commonly used as permeation barriers exhibited the least amount of volume and hardness change (<5%) when exposed to the test fuels. The response of other plastics (especially nylon) varied according to type and grade. Nylon 6 and Nylon 6,6 showed the lowest property changes following exposure Fuel C and the isobutanol blends, but swelled over 7% when exposed to CE25a. Acetal and polybutylene terephthalate (PBT) swelled around 5% with exposure to the test fuels, while high density polyethylene (HDPE) swelled around 10% for each test fuel. The remaining thermoplastics swelled to higher values and in the case of polypropylene, dissolution occurred with exposure to gasoline containing 25% ethanol. The fiberglass resins experienced more swelling in CE25a when compared to the baseline fuel or the two isobutanol blends. In general, the plastics exhibited a positive volume change when dried, which was attributed to fuel retention. For many plastics the Tg was not measurably affected by the test fuel exposures. However, polyethylene terephthalate (PET) and the nylons were notable exceptions. The Tg for PET was reduced by 30°C with CE25a, while the reductions observed for nylon depended on both nylon grade and oxygenate type.
Kass, Michael D.Janke, ChrisTheiss, TimothyPawel, SteveBaustian, JamesWolf, LesKoch, Wolf
The American Chemistry Council sponsored program to optimize a specimen design for use in high strain rate testing of long fiber-reinforced thermoplastics (LFRT) was experimentally validated through testing of injection molded long glass-filled polypropylene (LGFPP) and long glass filled Nylon ® (Nylon). It was demonstrated that the dynamic specimen geometry generated valid results for LFRT tensile tests in the quasi-static through 400/s regime. Optimum specimen size depended on the maximum test rates and end use of the data. The program results provide a basis to select specimen parameters to appropriately represent LFRT or similar materials for comparison or material property testing. Tests established the effects of injection technique; strain rate (nominal 0.1/s to 400/s); fiber fill content (20wt%, 30wt%, 40wt%), specimen type and width, panel thickness, distance to the fill gate, flow orientation, and material homogeneity. Not all variables were tested using material from both vendors. For a given LGFPP specimen size and vendor, the strength and modulus increased with fiber content, specimen width, and nominal strain rate. The LGFPP strength and failure strain increased between 0.001/s and 4/s but remained constant between 4/s and 45/s. Macroscopic and microscopic examinations of the fractures surfaces showed a strong mechanical bond between the fibers and the matrix. The Nylon demonstrated no difference in the strength between specimens identified with large or small amounts of fiber clusters. The ultimate strength, yield strength, and modulus of Nylon° increased between 0.001/s and 45/s. The failure strain decreased between 0.001/s and 45/s.
Kuhlman, Sarah J.H.Hill, Susan I.
Changes in the automotive supply chain over the past several years were brought about by global economic pressures, and forced some materials into tight supply as the industry started its recovery. One such material is polyamide 6,6 fiber (PA 6,6) used for airbags, which was in tight supply in 2008-09. This, with the availability of new low temperature inflators caused some airbag module manufacturers to revisit the use of polyester (PET), which had been used sporadically and in small quantities since the 1970s, although the overwhelming majority of airbags used PA 6,6. Over the last several years PET has been adopted for use in a small number of airbag programs to reduce supply concerns, but this use has come with performance tradeoffs of higher weight, lower tear and seam properties, and other changes. Still, the lower polymer cost of PET has driven a wider evaluation. Polyamide 6,6 and polyester are not equivalent fibers, and differences in thermal capacity, toughness, modulus, and other properties result in different fabric performance. The purpose of this paper is to raise awareness of key property differences so that the appropriate polymer is selected for each airbag. This report is a summary of studies conducted by INVISTA S.á.r.l. to understand the potential consequences and important considerations of changing airbag cushion material from polyamide 6,6 to polyester. INVISTA is a current supplier of PA 6,6 and PET for a wide range of products including airbags, and can thus provide an unbiased view on the materials. These studies include the analysis of airbag modules that changed from PA 6,6 to PET, and laboratory tests of fibers and fabrics measuring the performance differences between these polymers.
Orme, BradleyWalsh, Robert V.Westoby, Scott
The thermal efficiency of an internal combustion engine at steady state temperatures is typically in the region of 25-35%[1]. In a cold start situation, this reduces to be between 10% and 20% [2]. A significant contributor to the reduced efficiency is poor performance by the engine lubricant. Sub optimal viscosity resulting from cold temperatures leads to poor lubrication and a subsequent increase in friction and fuel consumption. Typically, the engine lubricant takes approximately twenty minutes [3] to reach steady state temperatures. Therefore, if the lubricant can reach its steady state operating temperature sooner, the engine's thermal efficiency will be improved. It is hypothesised that, by decoupling the lubricant from the thermal mass of the surrounding engine architecture, it is possible to reduce the thermal energy loss from the lubricant to the surrounding metal structure in the initial stages of warm-up. Using a bespoke oil flow rig described in the methodology section of this paper, it has been demonstrated that the addition of a 2 mm thick nylon tube, increases the maximum temperature differential between the lubricant and surrounding metal by 145% and reduces the energy losses from the gallery by 50%. This results from the addition of both a high thermal resistance material and a contact resistance between the polymer tube and metal. The insulating performance of nylon has been closely matched by utilising a specially designed aluminium insert with a 0.5 mm air gap. The increased contact resistance of such an insert has been shown to increase the temperature differential by 107% and reduce energy losses by 40%.
Roberts, Andrew P.Brooks, RichardShipway, PhilipGilchrist, RobertPegg, Ian
AE-8C2 Terminating Devices and Tooling Committee
The use of acoustic cavity fillers or “baffles” to prevent the propagation of air borne and structure borne noise, water and dust into the interior spaces of vehicle structures has been in practice for many years. Continuous development of new OEM requirements has pushed the state of the art concerning the design and functionality of these cavity sealing systems. Various technologies are available to OEMs to provide sealing that will prevent water and dust penetration, maximize performance of vehicle HVAC systems, and minimize the propagation of noise from the body structure into the interior compartment under operating conditions. Generally, three types of cavity sealing systems are available: pre-formed thermoplastic-based systems that incorporate a heat reactive thermoplastic sealer applied to a nylon or steel “carrier” for attachment to the body structure; heat reactive rubber-based sealer systems that incorporate a carrier, push pin or pressure sensitive adhesive layer for attachment; and bulk applied chemically reactive two component polyurethane or expandable “foam” systems. In this case study, a challenge undertaken by this supplier was to provide a thermoplastic baffle design of equal or lesser weight compared to a competitive, die-cut rubber-based technology currently in production at a particular OEM, while achieving equivalent acoustical performance. This paper will document the alternative design proposals and development activities that were pursued to meet this particular objective.
Fasse, MichaelBrichet, Nicolas
This SAE Standard covers complete general and dimensional specifications for tube fittings of the spherical and flanged sleeve compression types for use in the piping of air brake systems on automotive vehicles. The spherical sleeve compression type Figures 1A to 5 and Tables 1 to 3 is intended for use with annealed copper alloy tubing per SAE J1149, Type 1. The flanged sleeve compression type Figures 6A to 11 and Tables 4 to 6 is intended for use with nylon tubing per SAE J844. It is not intended to restrict or preclude other designs of a tube fitting for use with SAE J844, air brake tubing. Performance requirements for SAE J844 are covered in SAE J1131. See SAE J1131 for the Performance Requirements of Reusable (Push to Connect) Fittings Intended for Use in Automotive Air Brake Systems. CAUTION: To assure satisfactory performance, tapered sleeve compression type fitting components (SAE J512) should not be intermixed with the spherical or flanged sleeve components, nor should the spherical sleeve compression type components be intermixed with the flanged sleeve compression type components when assembling connection in areas where the three types are available.
Air Brake Tubing and Tube Ftg Committee
A resin coating was applied to a piston skirt for use in an internal combustion engine to reduce the frictional resistance on its surface. The purpose of the authors' study was to observe the change in surface states with the addition of nylon and graphite to the coating as solid lubricant particles in order to investigate the tribological properties of the surface. The authors observed self-formed microdimples on the resin surface when nylon particles were added to the polyamide-imide (PAI) coating material. These microdimples functioned as oil reservoirs similar in size to the nylon particles. The authors used PAI as a binder, and graphite particles (5 μm) and two different grades (5 and 10 μm) of nylon-12 particles as additives. These materials were mixed in a solvent, and an aluminum test sample was coated. The test sample was then heated in an oven to cure the PAI. Next, the texture of the surface was observed. The tribological properties were measured with a ball-on-disk tribometer under both oil lubrication and dry conditions. When only graphite particles were added to PAI, microdimples did not form on the surface of the coatings. However, the authors observed microdimples when both nylon and graphite particles were added. Sliding tests under oil lubrication showed a minimum value of the friction coefficient when 3-5 vol% of nylon was added. The addition of nylon particles to the graphite/PAI mixture decreased the friction coefficient at slow sliding speeds. Under the dry condition, the addition of a small amount of nylon did not affect the coefficient, but the friction coefficient decreased as the amount of graphite particles increased.
Suzuki, NobuyukiHikasa, Akio
Heat management with common textiles such as nylon and spandex is hindered by the poor thermal conductivity from the skin surface to cooling surfaces. This innovation showed marked improvement in thermal conductivity of the individual fibers and tubing, as well as components assembled from them.
Textile-based energy absorbers are under consideration for possible use as load-limiting devices for heavy payload tie-down systems in rotorcraft. In the event of a hard landing, these devices could prevent failure of the mounting system and subsequent uncontrolled motion of the payload. A series of environmental conditioning regimens were imposed on the textile load limiters, which are polyester tear webbings and nylon stitch-ripping devices. These test specimens were exposed to: ambient conditions; salt-fog spray; isopropyl alcohol; hydraulic fluid; hot-water immersion; kerosene; and either high or low temperatures. The results, based on performance measures of: specific energy absorption, volumetric energy absorption, linear energy absorption, and coefficient of variation of force, demonstrated that the high temperature conditioning caused the most prominent decrease in performance while the other conditions showed only small variations. Both devices were also tested at rates as high as 15 m/s in ambient conditions. The devices were found to have only a slight reduction in performance under dynamic testing conditions versus quasi-static conditions.
Miller, SimonBakis, CharlesSmith, EdwardLittle, EricYukish, Michael
The material defined by this SAE document is an impact modified, heat stabilized, 66 nylon reinforced with glass fibers. This material is for use in dust shields for hydraulic disc brakes. NOTE—The applicability of a plastic dust shield must be evaluated for each individual brake system. Its use with solid rotors and/or high performance brake systems is not recommended.
Hydraulic Brake Components Standards Committee
The growing use of bio-based fuels today has created new performance and design considerations for high-performance polyamides used in a range of automotive fuel components such as fuel rails, diesel fuel filter housings, fuel sender units, flanges, fuel connectors, and quick connectors. During the material selection process, engineers need to take into account not only the basic tenets of metal-to-plastic conversion, but also the type of fuel and its impact on the performance of the materials. Conventional gasoline is being modified with aliphatic alcohols such as ethanol and methanol. In the U.S., the percentage of alcohol ranges up to 85% (E85) while in Brazil the usage of 100% ethanol (E100) is typical. Also, diesel fuel can be replaced by 100% of biodiesel sourced from sustainable resources such as soy, rape seed, sugar cane, and animal grease. In Brazil, B100 biodiesel (100% biodiesel content) isn't ready for commercial use. Currently, B5 (5% biodiesel content) is regulated for commercial use while in the U.S. and Europe auto makers are designing for components that use B20 (20% biodiesel) added to regular diesel and in some cases B30 (30% biodiesel). These bio-based fuels can have an adverse effect on the long-term performance of aliphatic polyamides such as nylon 6, nylon 66, and nylon 12. However, semi-aromatic polyamides such as polyphthalamide (PPA) have demonstrated superior performance in these bio-fuel applications, retaining their properties over the long term. Bio-based fuels can cause swelling in parts made of nylon 66, resulting in significant dimensional changes and weight gain. In addition, the alcohol's oxygen content can break down the carbon-carbon bond in the PA 66 backbone, resulting in a loss of mechanical properties such as tensile strength. Similarly, in biodiesel applications, parts made of aliphatic polyamides are significantly affected by the presence of corrosive water that can cause severe chemical attack to the polymers. Ultimately, this could lead to leaks and failures in certain applications. Based on extensive testing and commercial use, higher performing semi-aromatic nylons such as PPA offer major advantages over aliphatic nylons, delivering superior chemical resistance, lower water absorption, and better dimensional stability. They offer the most favorable performance in critical fuel component applications, retaining mechanical performance after over 5000 hours of exposure. This paper will present property comparisons and design recommendations for high-performance polyamides for bio-based fuel applications.
Baleno, BrianBenjamin, EdgarDesai, KiritNorfolk, LindaCarvalho, Andre
For several decades, aircrew working within rotary wing aircraft and some cargo aircraft (C-130) have used a simple nylon Crewmembers Aircraft Safety Belt (CASB) with an adjustable tether length, commonly referred to as a “gunner’s belt,” as their fall protection system. The CMARS AIRSAVE interface, in conjunction with either the CMARS or MARS webbing retractor, will eliminate the CASB in an effort to increase fall and crash protection. This paper discusses the U.S. Navy development of a system that provides a substantial decrease in injury loads while significantly increasing fall and crash protection. The system utilizes the lifting harness already worn as part of the AIRSAVE survival vest, thus distributing the crash or fall loads over the aircrew member’s body. This paper will also discuss the design development from initial concept to prototyping, testing, and demonstration of the CMARS AIRSAVE interface in preparation for final introduction into the Fleet.
Sample, AngelaSmith, Jason
Seat Belt Entanglement in Rollover Accidents: Physical Evidence and Occupant Kinematics2008-01-12374/14/2008
In rollover accidents, physical evidence of seat belt usage is occasionally difficult to discern. Typically, if a seat belt is used by an occupant in an accident, various seat belt components will display characteristic marks in well-defined locations. These marks are known as “witness marks” or “occupant load marks.” Witness marks in a rollover accident may be faint in comparison to those caused by the occupant restraint forces in high-energy planar collisions. Additionally, in situations where a seat belt buckle is alleged to have unlatched early in a rollover accident, the lack of clear occupant load marks may in some cases be attributed to an alleged “buckle release” that occurred very early in the rollover sequence, so that the seat belt did not sustain loading while in a latched condition. However, a documented Case Study and preliminary testing indicate that release of a seat belt buckle during a rollover accident leads to entanglement of the occupant's torso and/or outboard arm in the webbing. This entanglement produces distinctive evidence on the seat belt assembly and vehicle, as well as injury to the occupant. To further evaluate occupant load marks unique to entanglement, dolly rollover tests were performed using a vehicle with a reinforced roof. Hybrid III Anthropomorphic Test Devices (ATDs) were seated in the front outboard seats with their respective seat belt tongues connected to their buckles using nylon cable ties to produce a simulated “buckle unlatching” very early in the rollover event. This testing showed that if the roll rate was high enough to produce occupant ejection, both driver and passenger-side occupants became entangled in the unlatched seat belts during ejection from the vehicle. This entanglement created occupant load marks substantially different from typical occupant restraint evidence, with a characteristic pattern observed on the vehicle and seat belt.
Raasch, ChristineDavee, DanielLuepke, Peter
STRATEGIES FOR AUTOMOBILE GEAR MATERIAL SELECTION2008-28-00551/9/2008
Material selection is based on Process such as forging, die-casting, machining, welding and injection moulding and application as type of load for Knife Edges and Pivots, to minimize Thermal Distortion, for Safe Pressure Vessels, Stiff, High Damping Materials, etc. In order for gears to achieve their intended performance, durability and reliability, the selection of a suitable gear material is very important. High load capacity requires a tough, hard material that is difficult to machine; whereas high precision favors materials that are easy to machine and therefore have lower strength and hardness ratings. Gears are made of variety of materials depending on the requirement of the machine. They are made of plastic, steel, wood, cast iron, aluminum, brass, powdered metal, magnetic alloys and many others. The gear designer and user face a myriad of choices. The final selection should be based upon an understanding of material properties and application requirements. This paper commences with a general overview of the methodologies of proper gear material selection to improve performance with optimize cost (including of design & process), weight and noise. We have materials such as SAE8620, 20MnCr5, 16MnCr5, Nylon, Aluminium, etc. used on Automobile gears. We have process such as Hot & cold forging, rolling, etc. This paper will also focus on uses of Nylon gears on Automobile as Speedo-gears and now moving towards the transmission gear by controlling the backlash. It also has strategy of gear material cost control.
Shastri, DilipRamamurthy, S.Parab, Pratap
More than twenty years have passed since we invented polymer-clay nanocomposites (PCN), in which only a few wt.-% of silicate is randomly and homogeneously dispersed in the polymer matrix. When molded, these nanocomposites show superior properties compared to pristine polymers such as tensile strength, tensile modulus, heat distortion temperature, gas barrier property, and so on. The number of papers on PCN has increased rapidly in recent years, reaching over 500 only in 2005. As the pioneers of the new technology, we will review its history highlighting our works. Epoch-making events of PCN are as follows: In 1985, The first PCN, nylon 6-clay hybrid (NCH), was invented. In 1987, NCH was first presented at the ACS Fall Meetings. In 1989, NCH was presented at the MRS Fall Meetings, firing PCN. In 1989, Toyota launched cars equipped with a NCH part. In 1996, Clay was found to cause a memory effect in liquid crystals. In 1997, Gilman of NIST et al. found revolutionary fire retardency in NCH. In 1997, PP-clay nanocomposite was prepared. In 1998, Compounding method for producing NCH was established. In 2002, Haraguchi of Kawamura Institute of Chemical Research et al. invented a nanocomposite hydrogel. So far only nylon-clay nanocomposites are used in practice, but other PCN will become increasingly useful in the future.
Okada, AkaneUsuki, Arimitsu
Research Work for the Improvement of the Durability of Glass Fiber-Reinforced Nylon 66 by Modifying the Glass Fiber Diameter2006-32-003211/13/2006
As for the polyamide (nylon) resins, i.e., nylon 6, nylon 66, nylon 46 and so on, when they are reinforced by glass fibers (GF), their static mechanical strength and heat distortion temperature increase considerably, and many faults of them are improved. However, when repeating stress is applied to a GF-reinforced nylon, the interface stress concentration between nylon and GF is easily to happen and so, depending upon working condition, the damage phenomenon similar to fatigue flaking is often observed for the GF-reinforced nylon by the reason of the insufficiency of interface strength between nylon and GF. In this study, thus, it mainly focused on the improvement of the fatigue property of GF-reinforced nylon. Actually, we compounded of nylon 66 and GF the fiber diameter of which was smaller than conventional GF, and investigated the mechanical and physical properties of the nylon 66 / GF composite we prepared. As a result, it was recognized that the fatigue property of the nylon 66 reinforced by GF the fiber diameter of which was 6μm was improved compared to nylon 66 reinforced by ordinary GF whose diameter was 13μm. In addition, it was revealed that the values of static mechanical strength and impact strength of the composite consisting of nylon 66 and GF having the diameter of 6μm also increased in comparison with a conventional GF-reinforced nylon 66. Moreover, a good result with respect to the evaluation of high temperature oxidation stability was obtained for the nylon 66 reinforced by GF having the diameter of 6 μm. Our developed material based on nylon 66 / the modified GF composite has the properties that permit applying our new nylon / GF composite to the material used for the reduction gear of the Electric Power Steering (EPS) system used under severe condition.
Murakami, TakeshiTakajo, Toshimi
Analysis of the Deterioration of Nylon-66 Immersed in GTL Diesel Fuel Part 2. Analysis of Model Fuel and Nylon Before and After Immersion2006-01-332710/16/2006
In a previous paper (Part 1 of this series), nylon-66 specimens were immersed in two GTL diesel fuels (GTL-A and GTL-B) and then subjected to tensile testing. The tensile test results revealed that the elongation of the specimen immersed in GTL-A was dramatically reduced. The GTL diesel fuels and nylon specimens before and after immersion were analyzed to determine the cause of the decline in elongation. It was found that the poor elongation was caused by penetration and oxidation of low molecular-weight paraffins and that the ease of penetration and oxidation of paraffin depended on the structure of paraffin. In this paper, the low molecular-weight paraffins detected in GTL-A were mixed to produce model fuels. Then, pieces of nylon cut from the tensile test specimen, were immersed in the model fuels. In addition, partial oxidation products of the paraffin (alcohol, aldehyde or ketone and acid) were used in immersion tests of the nylon pieces. It was found that: (1) The quaternary carbon atom in i-paraffin hardly oxidizes, while the tertiary carbon atom in i-paraffin readily oxidizes to give alcohol. (2) 2-Methyl-paraffin produced 100 times as many oxidation products as n-paraffin. (3) The lower the carbon number of a paraffin is, the easier it penetrates the nylon samples. (4) The degree of oxidation of nylon corresponded with the tendency of paraffin to oxidize. (5) The composition of the oxidation products of paraffin, which were detected in the nylon after the immersion test, was nearly the same as that of the oxidation products of paraffin itself. (6) Oxidation products of the paraffin outside of the nylon had no influence on the oxidation of the inner layer of nylon. Rather, the free radicals that oxidized the inner layer of nylon were generated from the paraffin that entered the nylon.
Ogawa, TadaoOhshima, AyakoNakai, KyokoOkamoto, KazuoMurase, AtsushiHayashi, Hitoshi
Analysis of the Deterioration of Nylon-66 Immersed in GTL Diesel Fuel Part 1. Analysis and Test of Nylon and GTL Diesel Fuel Before and After Immersion2006-01-332610/16/2006
The effect of GTL diesel fuel on organic materials used in fuel delivery systems of vehicles was investigated. Specimens made from 16 kinds of organic materials were immersed in GTL diesel fuels synthesized at Refinery-A and Refinery-B (referred to as GTL-A and GTL-B, respectively) and then subjected to tensile testing. The tensile test results revealed that elongation of the nylon sample immersed in GTL-A was extremely small, about 4% of that of untreated nylon. In the light of this finding, the GTL diesel fuels and nylons before and after immersion test were analyzed in detail using about 20 analysis methods to determine the cause for poor elongation. The following points were found. (1) GTL-A consisted of low molecular-weight paraffins. (2) GTL-A had low molecular-weight i-paraffins. (3) The nylon immersed in GTL-A contained low molecular-weight paraffins. (4) The paraffins in the nylon immersed in GTL-A were richer in i-paraffins than the original GTL-A. From previous experiments using model fuel, it was found that i-paraffins penetrate nylon and oxidize more rapidly in the nylon than n-paraffins. (5) The nylon immersed in GTL-A was oxidized from the surface to a depth of 400 μm. (6) i-Paraffins produced about 100 times as many oxidation products as n-paraffins. From these results, it was concluded that the low molecular-weight paraffins in GTL-A penetrated the nylon and caused it to swell. These paraffins oxidized in the nylon and became free radicals, which then oxidized and depolymerized the nylon molecules. This depolymerization of the nylon caused the poor elongation as a result of the dissociation of hydrogen bonds between the nylon molecules.
Ogawa, TadaoKajiya, SyujiOhshima, AyakoMurase, AtsushiSuzuki, YasuyukiHayashi, Hitoshi
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